Soy muy nuevo con JSON, ¡por favor ayuda!

Estoy tratando de serializar unList<KeyValuePair<string, string>> como JSON

Actualmente:

[{"Key":"MyKey 1","Value":"MyValue 1"},{"Key":"MyKey 2","Value":"MyValue 2"}]

Esperado:

[{"MyKey 1":"MyValue 1"},{"MyKey 2":"MyValue 2"}]

Me referí a algunos ejemplos deesta yesta.

Este es mi KeyValuePairJsonConverter: JsonConverter

public class KeyValuePairJsonConverter : JsonConverter
{
    public override void WriteJson(JsonWriter writer, object value, JsonSerializer serializer)
    {
        List<KeyValuePair<object, object>> list = value as List<KeyValuePair<object, object>>;
        writer.WriteStartArray();
        foreach (var item in list)
        {
            writer.WriteStartObject();
            writer.WritePropertyName(item.Key.ToString());
            writer.WriteValue(item.Value.ToString());
            writer.WriteEndObject();
        }
        writer.WriteEndArray();
    }

    public override bool CanConvert(Type objectType)
    {
        return objectType == typeof(List<KeyValuePair<object, object>>);
    }

    public override object ReadJson(JsonReader reader, Type objectType, object existingValue, JsonSerializer serializer)
    {
        var jsonObject = JObject.Load(reader);
        var target = Create(objectType, jsonObject);
        serializer.Populate(jsonObject.CreateReader(), target);
        return target;
    }

    private object Create(Type objectType, JObject jsonObject)
    {
        if (FieldExists("Key", jsonObject))
        {
            return jsonObject["Key"].ToString();
        }

        if (FieldExists("Value", jsonObject))
        {
            return jsonObject["Value"].ToString();
        }
        return null;
    }

    private bool FieldExists(string fieldName, JObject jsonObject)
    {
        return jsonObject[fieldName] != null;
    }
}

Lo llamo desde un método de WebService como este

List<KeyValuePair<string, string>> valuesList = new List<KeyValuePair<string, string>>();
Dictionary<string, string> valuesDict = SomeDictionaryMethod();

foreach(KeyValuePair<string, string> keyValue in valuesDict)
{
    valuesList.Add(keyValue);
}

JsonSerializerSettings jsonSettings = new JsonSerializerSettings { Converters = new [] {new KeyValuePairJsonConverter()} };
string valuesJson = JsonConvert.SerializeObject(valuesList, jsonSettings);